A team of researchers at Politecnico di Milano, University Grenoble Alpes and other institutes worldwide have recently demonstrated the non-volatile control of the spin-to-charge conversion in germanium telluride, a known Rashba semiconductor, at room temperature. Their work could have important implications for the future development of spintronic devices.

The Rashba effect, discovered in 1959, entails a momentum-independent splitting of spin bands in two-dimensional condensed matter systems. In ferroelectric Rashba semiconductors, this effect can be reversed by switching the direction of the ferroelectric polarization. The idea that Rashba spin-splitting in these materials can be controlled was confirmed by a series of first-principle calculations by S. Picozzi and later validated in spectroscopic experiments using germanium telluride, which is thus often considered the 'prototype' of the ferroelectric Rashba class of semiconductors.

To demonstrate the ferroelectric control of the spin-to-charge conversion, Rinaldi and his colleagues first had to show that controlling ferroelectricity in germanium telluride by applying voltage pulses to metallic contacts deposited on the semiconductor was possible. Subsequently, they injected spin-currents into germanium telluride and measured the resulting charge current, comparing it to the polarization state.

"We demonstrated the ferroelectric gating of the semiconductor by applying voltage pulses through a thin metallic gate on top of germanium telluride," Sara Varotto, a Ph.D. researcher who carried out the study, explained. "We mapped the distribution of ferroelectric domains underneath the gate using the conductive tip of an atomic force microscope. We also discovered a link between the ferroelectric domains configuration and the electric resistance of metal/germanium telluride junctions, a very effective way to easily access to the polarization state."

Varotto subsequently performed a series of spin pumping experiments at University Grenoble Alpes, under the supervision of researchers Laurent Vila and Jean-Philippe Attané. The team excited an iron layer in contact with the germanium telluride sample to inject a spin current into the semiconductor. These experiments revealed that spinning electrons are deflected to the left or right by germanium telluride, depending on the direction of the ferroelectric polarization.

"We reveal that spin Hall effect is responsible for this conversion from spin to charge currents in germanium telluride, thanks to the precious work of Jagoda Slawinska and Marco Buongiorno Nardelli from University of North Texas," Rinaldi said. "A similar non-volatile electric control of spin-charge conversion has also been demonstrated in oxides-based two-dimensional electron gas. A very significant discovery, so far limited by the fact that the system works at cryogenic temperatures, in materials potentially difficult to integrate on silicon."



This team of researchers is the first to demonstrate ferroelectric switching of the spin-to-charge conversion at room temperature in a semiconductor that could be monolithically integrated on silicon.

"We also proposed a conceptual logic device that shares the favorable scaling law and low power consumption with Intel's MESO device, but with a great overall simplification offered by the fact that germanium telluride has both memory and spin transduction capabilities in the same material, thereby eliminating complex solutions to write the information," Rinaldi said. "Similarly to what happens in our brain, the memory and the computation reside in the same physical space, with perspectives in in-memory computing."

In the future, the strategy for controlling spin-to-charge conversion in germanium telluride proposed by Rinaldi and his colleagues could be applied to the development of new spintronic devices. Moreover, as the device they theoretically proposed in their paper can store and process information in the same physical space, similarly to the human brain, it could prove particularly useful for in-memory computing applications.

"My research focuses on spin-based solutions in novel quantum materials to help the development of a new computing era," Rinaldi added. "The first step in this sense will comprise material engineering of ferroelectric Rashba semiconductors to bring such compound much closer to technology."

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